Seikei-Kakou
Online ISSN : 1883-7417
Print ISSN : 0915-4027
ISSN-L : 0915-4027
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Index
Foreword
Technical Notes : Special Issue on Biomedical Polymers -Development, Safety and Regulation-
Special Lecture "Polymer Processing : Bridge to the Future"
Technical Reports
Report of Meetings and Trade Fair
Original Papers
  • Kosaku Tao, Seiji Higashi, Keitaro Kago, Koji Yamada
    2025 Volume 37 Issue 6 Pages 255-259
    Published: May 20, 2025
    Released on J-STAGE: June 20, 2025
    JOURNAL FREE ACCESS

    In this study, we investigated the relationship between amorphous structure and physical heat resistance in polylactic acid (PLA) injection moldings. When the amorphous PLA moldings underwent heat treatment at a temperature below the glass transition temperature (Tg), the heat distortion temperature (HDT) increased without cold crystallization. Also, we clarified that there is an optimum heat treatment temperature in terms of the increase in HDT. Comparing heat treatment temperature dependence of the increase in HDT and enthalpy relaxation, we concluded that the increase in HDT of the amorphous PLA moldings due to the heat treatment below Tg is related to enthalpy relaxation. Also, we investigated the effect of heat treatment on HDT in the PLA injection moldings after cold crystallization. The heat treatment also relieved excess enthalpy in the crystalline PLA moldings. Furthermore, the segmental motion associated with α - relaxation in the crystalline PLA moldings was suppressed to the same extent as in the amorphous PLA moldings, but the degree of increase in HDT due to the heat treatment was much smaller than in the case of amorphous PLA moldings. On the other hand, comparison of the deflection curves before and after the heat treatment revealed that the temperature at which the amount of distortion in HDT begins to increase was greatly raised by the heat treatment in the crystalline PLA moldings.

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